Matches in SemOpenAlex for { <https://semopenalex.org/work/W3022118226> ?p ?o ?g. }
- W3022118226 endingPage "23903" @default.
- W3022118226 startingPage "23896" @default.
- W3022118226 abstract "The development of high-performance, low-cost, and long-lasting electrocatalysts for both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is urgently needed for effective electrochemical water splitting. In the present study, an engineering process was employed to prepare Lewis base-hungry amorphous-crystalline nickel borate-nickel sulfide (Ni3(BO3)2-Ni3S2) heterostructures, which exhibited unprecedentedly high electrocatalytic activity toward both OER and HER in alkaline media. The optimal Ni3(BO3)2-Ni3S2/nickel foam (Ni3(BO3)2-Ni3S2/NF) electrode displayed an ultralow overpotential of only -92 and +217 mV to reach the current density of 10 mA cm-2 for HER and OER, respectively. When the Ni3(BO3)2-Ni3S2/NF electrode was used as both the anode and cathode for overall water splitting, a low cell voltage of 1.49 V was needed to achieve the current density of 10 mA cm-2, which was superior to the performance of most noble metal-free electrocatalysts. Results from density functional theory calculations showed that the Lewis base-hungry sites in the heterostructures effectively enhanced the chemisorption of hydrogen and oxygen intermediates, a critical step in HER and OER electrocatalysis. Results from this study highlight the significance of rational design and engineering of heterostructured materials for the development of high-efficiency electrocatalysts." @default.
- W3022118226 created "2020-05-13" @default.
- W3022118226 creator A5002654282 @default.
- W3022118226 creator A5008007560 @default.
- W3022118226 creator A5010534418 @default.
- W3022118226 creator A5011687434 @default.
- W3022118226 creator A5013444381 @default.
- W3022118226 creator A5023844763 @default.
- W3022118226 creator A5028960226 @default.
- W3022118226 creator A5033273196 @default.
- W3022118226 creator A5046662106 @default.
- W3022118226 creator A5047179940 @default.
- W3022118226 creator A5051630707 @default.
- W3022118226 creator A5069739391 @default.
- W3022118226 date "2020-05-04" @default.
- W3022118226 modified "2023-10-13" @default.
- W3022118226 title "“Lewis Base-Hungry” Amorphous–Crystalline Nickel Borate–Nickel Sulfide Heterostructures by In Situ Structural Engineering as Effective Bifunctional Electrocatalysts toward Overall Water Splitting" @default.
- W3022118226 cites W1982414605 @default.
- W3022118226 cites W1997046539 @default.
- W3022118226 cites W2014788410 @default.
- W3022118226 cites W2022714449 @default.
- W3022118226 cites W2032100925 @default.
- W3022118226 cites W2070469412 @default.
- W3022118226 cites W2087059155 @default.
- W3022118226 cites W2091875228 @default.
- W3022118226 cites W2159202183 @default.
- W3022118226 cites W2201339550 @default.
- W3022118226 cites W2287479925 @default.
- W3022118226 cites W2323587486 @default.
- W3022118226 cites W2337711932 @default.
- W3022118226 cites W2461202500 @default.
- W3022118226 cites W2512398054 @default.
- W3022118226 cites W2558658892 @default.
- W3022118226 cites W2588882602 @default.
- W3022118226 cites W2623419721 @default.
- W3022118226 cites W2752366461 @default.
- W3022118226 cites W2756623587 @default.
- W3022118226 cites W2794092806 @default.
- W3022118226 cites W2796364604 @default.
- W3022118226 cites W2801361960 @default.
- W3022118226 cites W2807764879 @default.
- W3022118226 cites W2883061945 @default.
- W3022118226 cites W2886581020 @default.
- W3022118226 cites W2891942906 @default.
- W3022118226 cites W2892890167 @default.
- W3022118226 cites W2898876180 @default.
- W3022118226 cites W2900054010 @default.
- W3022118226 cites W2903890094 @default.
- W3022118226 cites W2904432893 @default.
- W3022118226 cites W2904657824 @default.
- W3022118226 cites W2909007076 @default.
- W3022118226 cites W2914544678 @default.
- W3022118226 cites W2920270139 @default.
- W3022118226 cites W2920893142 @default.
- W3022118226 cites W2929386906 @default.
- W3022118226 cites W2963997550 @default.
- W3022118226 cites W2965820860 @default.
- W3022118226 cites W2967299079 @default.
- W3022118226 cites W2981290216 @default.
- W3022118226 cites W2986755912 @default.
- W3022118226 doi "https://doi.org/10.1021/acsami.0c03796" @default.
- W3022118226 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32362112" @default.
- W3022118226 hasPublicationYear "2020" @default.
- W3022118226 type Work @default.
- W3022118226 sameAs 3022118226 @default.
- W3022118226 citedByCount "46" @default.
- W3022118226 countsByYear W30221182262020 @default.
- W3022118226 countsByYear W30221182262021 @default.
- W3022118226 countsByYear W30221182262022 @default.
- W3022118226 countsByYear W30221182262023 @default.
- W3022118226 crossrefType "journal-article" @default.
- W3022118226 hasAuthorship W3022118226A5002654282 @default.
- W3022118226 hasAuthorship W3022118226A5008007560 @default.
- W3022118226 hasAuthorship W3022118226A5010534418 @default.
- W3022118226 hasAuthorship W3022118226A5011687434 @default.
- W3022118226 hasAuthorship W3022118226A5013444381 @default.
- W3022118226 hasAuthorship W3022118226A5023844763 @default.
- W3022118226 hasAuthorship W3022118226A5028960226 @default.
- W3022118226 hasAuthorship W3022118226A5033273196 @default.
- W3022118226 hasAuthorship W3022118226A5046662106 @default.
- W3022118226 hasAuthorship W3022118226A5047179940 @default.
- W3022118226 hasAuthorship W3022118226A5051630707 @default.
- W3022118226 hasAuthorship W3022118226A5069739391 @default.
- W3022118226 hasConcept C127413603 @default.
- W3022118226 hasConcept C135473242 @default.
- W3022118226 hasConcept C147789679 @default.
- W3022118226 hasConcept C161790260 @default.
- W3022118226 hasConcept C17525397 @default.
- W3022118226 hasConcept C179104552 @default.
- W3022118226 hasConcept C185592680 @default.
- W3022118226 hasConcept C186460083 @default.
- W3022118226 hasConcept C191897082 @default.
- W3022118226 hasConcept C192562407 @default.
- W3022118226 hasConcept C2780443040 @default.
- W3022118226 hasConcept C2780596425 @default.
- W3022118226 hasConcept C2781281706 @default.
- W3022118226 hasConcept C33989665 @default.
- W3022118226 hasConcept C35590869 @default.