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• W3022172078 abstract "Low-dimensional organic-inorganic hybrid materials have attracted tremendous attentions due to their fascinating properties as emerging star materials for light-emitting applications. Taking advantage of their rich chemical composition and structural diversity, here, a novel lead-free organic-manganese halide compound, (1-mPQBr)2MnBr4 (1-mPQ=1-methylpiperazine, 1-C5H14N2) with zero-dimensional structure has been rationally designed and successfully synthesized through solvent-evaporation method. Systematical characterizations were carried out to investigate the structure, thermal and photophysical properties. The (1-mPQBr)2MnBr4 was found to crystallized into an orthorhombic crystal (P212121) with lattice parameters of a=8.272(6) Å, b=15.982(10) Å and c=17.489(11) Å. The structure consists of isolated [MnBr4]2- clusters and free Br- ions as well as [C5H14N2]2+ molecules. Thermal analysis indicates that it is stable up to 300 °C. Upon ultraviolet photoexcitation, the (1-mPQBr)2MnBr4 exhibits intense green emission centered at 520 nm with a narrow full width at half-maximum of 43 nm at room temperature, which should be assigned to the spin-forbidden internal transition (4T1(G) to 6A1) of tetrahedrally coordinated Mn2+ ions. The superior photoluminescence properties coupled with facile and efficient synthesis method of this material suggest its considerable promise to be utilized as light-emitting materials." @default.
• W3022172078 created "2020-05-13" @default.
• W3022172078 creator A5011598568 @default.
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• W3022172078 date "2020-04-28" @default.
• W3022172078 modified "2023-10-18" @default.
• W3022172078 title "(1-C5H14N2Br)2MnBr4: A Lead-Free Zero-Dimensional Organic-Metal Halide With Intense Green Photoluminescence" @default.
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• W3022172078 doi "https://doi.org/10.3389/fchem.2020.00352" @default.
• W3022172078 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7199156" @default.
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