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- W3022355951 abstract "As the kinetically sluggish oxygen evolution reaction (OER) is considered to be a bottleneck in overall water splitting, it is necessary to develop a highly active and stable electrocatalyst to overcome this issue. Herein, we successfully fabricated a three-dimensional iron-dysprosium oxide co-regulated in-situ formed MOF-Ni arrays on carbon cloth ([email protected]/CC) through a facile two-step hydrothermal method. Electrochemical studies demonstrate that the designed [email protected]/CC catalyst requires an overpotential of only 251 mV to reach 10 mA cm−2 with a small Tafel slope of 52.1 mV dec−1. Additionally, the stability declined by only 5.5% after 80 h of continuous testing in 1.0 M KOH. Furthermore, a cell voltage of only 1.57 V in the overall water splitting system is sufficient to achieve 10 mA cm−2; this value is far better than that of most previously reported catalysts. The excellent catalytic performance originates from the unique 3D rhombus-like structure, as well as coupling synergies of Fe-Dy-Ni species. The combination of lanthanide and transition metal species in the synthesis strategy may open entirely new possibilities with promising potential in the design of highly active OER electrocatalysts." @default.
- W3022355951 created "2020-05-13" @default.
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- W3022355951 date "2020-11-01" @default.
- W3022355951 modified "2023-10-12" @default.
- W3022355951 title "Dissolution-regrowth of hierarchical Fe-Dy oxide modulates the electronic structure of nickel-organic frameworks as highly active and stable water splitting electrocatalysts" @default.
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- W3022355951 doi "https://doi.org/10.1016/s1872-2067(20)63606-3" @default.
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