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• W3022775810 abstract "The science and technology of intercalation compounds developed in the project “Carbon Alloys” are summarized in this chapter. The subjects are: lithium insertion into carbon materials, new intercalation compounds prepared from unique host carbon materials, and host effects following the intercalation of halogen molecules and alkali metals. Several carbons are examined as possible anodes of lithium-ion batteries and the origins of large capacities of less graphitized carbons are debated. Theoretical approaches are proposed for the analysis and design of anode materials with high performances. Effects of heteroatoms introduced into carbons have been extensively investigated by experiment and by calculation. The electronic and magnetic properties of diamond-derived nanographite and its derivatives formed by the intercalation of potassium and halogen molecules are investigated. It was found that edge-inherited non-bonding π-electron states play an essential role in characterizing the electronic structure of nanographite. The intercalation of potassium into nanographite diminishes the contribution of the edge-states due to charge transfer from the potassium atom. Evidence of charge transfer from nanographite to iodine, absent in bulk-graphite, is identified. The charge transfer fraction, per carbon atom fc, follows the order of potassium > bromine > iodine. Intercalation of cesium into carbon materials with different heat-treatment temperatures (HTT) was carried out and the resultant carbon alloys were characterized by XRD, ESR, Raman spectroscopy and molecular sorption techniques. Increases in carbon–carbon interlayer spacings due to intercalation by cesium were observed even for less-graphitized carbons of HTT < 1273 K. The compound CsC24 was able to sorb molecules such as hydrogen, although almost no shift of the Raman peak (G-band) was observed, suggesting weak interactions between the cesium and carbon layers." @default.
• W3022775810 created "2020-05-13" @default.
• W3022775810 creator A5035331820 @default.
• W3022775810 date "2003-01-01" @default.
• W3022775810 modified "2023-09-23" @default.
• W3022775810 title "Intercalation Compounds" @default.
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• W3022775810 doi "https://doi.org/10.1016/b978-008044163-4/50006-1" @default.
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