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• W3022974134 abstract "ConspectusNitroxyl (HNO) is a biological signaling agent that displays distinctive reactivity compared to nitric oxide (NO). As a consequence, these two reactive nitrogen species trigger different physiological responses. Selective detection of HNO over NO has been a challenge for chemists, and several fluorogenic molecular probes have been recently developed with that goal in mind. Common constructs take advantage of the HNO-induced reduction of Cu(II) to Cu(I). The sensing mechanism of such probes relies on the ability of the unpaired electron in a d orbital of the Cu(II) center to quench the fluorescence of a photoemissive ligand by either an electron or energy transfer mechanism. Experimental and theoretical mechanistic studies suggest that proton-coupled electron transfer mediates this process, and careful tuning of the copper coordination environment has led to sensors with optimized selectivity and kinetics.The current optical probes cover the visible and near-infrared regions of the spectrum. This..." @default.
• W3022974134 created "2020-05-13" @default.
• W3022974134 creator A5023547067 @default.
• W3022974134 creator A5034625027 @default.
• W3022974134 date "2015-11-01" @default.
• W3022974134 modified "2023-09-27" @default.
• W3022974134 title "Metal-Based Optical Probes for Live Cell Imaging of Nitroxyl (HNO)" @default.
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• W3022974134 hasPublicationYear "2015" @default.
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