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- W3023406147 abstract "It is essential mean to adsorptive remove organic pollutants such dyestuff for water remediation. Herein in situ modification of the classic metal-organic framework ZIF-67 with –SO3− groups was easily achieved by the efficient adsorption of multi-sulfonated dyes due to the coordinative interaction between the unoccupied Co(II) of ZIF-67 and –SO3− of the dyes. Interestingly, highly efficient synergistic absorption of multi-sulfonated dyes towards methylene blue (MB+) upon ZIF-67 was discovered for the first time. The improved adsorption capacity of ZIF-67 for MB+ in presence of cotton blue (CB−) was measured with a record-high value of 5,857.9 mg/g. The underlying mechanism of the synergistic adsorption was probed, showing that, after the initial coordination between the –SO3− of the dyes and the unoccupied Co(II) of ZIF-67, the available –SO3− groups of multi-sulfonated dyes can interact with –N+(CH3)2 in MB+ and hence greatly improving the adsorption capacity of MB+." @default.
- W3023406147 created "2020-05-13" @default.
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- W3023406147 date "2020-08-01" @default.
- W3023406147 modified "2023-10-15" @default.
- W3023406147 title "In situ modification of ZIF-67 with multi-sulfonated dyes for great enhanced methylene blue adsorption via synergistic effect" @default.
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- W3023406147 doi "https://doi.org/10.1016/j.micromeso.2020.110304" @default.
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