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• W3024211282 startingPage "2242" @default.
• W3024211282 abstract "A new strategy is reported to improve the performance of BaZrO3-based protonic ceramic conductors by substitution on the anion sublattice, specifically replacing F− in the O2− site. The F−-doped material exhibited higher conductivity under both reducing and oxidizing atmospheres compared to the undoped oxide. Ab initio calculations and X-ray photoelectron spectroscopy results showed that the improved performance can be attributed to weakened chemical bonding between the cations (A or B site) and the oxygen ions as a result of F− doping, resulting in improved oxygen mobility. Finally, improved performance was demonstrated by using BaZr0.8Y0.2O3-δ-σFσ (σ=0.1) as the electrolyte in protonic ceramic fuel cells measurements. The anions doping strategy shows great promise for the development of a new generation of high-performance electrolyte materials." @default.
• W3024211282 created "2020-05-21" @default.
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• W3024211282 date "2020-04-14" @default.
• W3024211282 modified "2023-10-17" @default.
• W3024211282 title "Fluoride‐Based Anion Doping: A New Strategy for Improving the Performance of Protonic Ceramic Conductors of the Form BaZrO ₃" @default.
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• W3024211282 doi "https://doi.org/10.1002/celc.202000154" @default.
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