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- W3025232304 endingPage "119118" @default.
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- W3025232304 abstract "Methane, a highly abundant greenhouse gas with a high global warming potential, is a relatively clean fuel due to its high H/C ratio. This study has taken a unique approach to discover key fundamentals during the solution combustion synthesis of Pd0.03Ce0.97O2-δ catalysts characterised using several physicochemical techniques for catalytic CH4 combustion. Oxygen vacancies were found to be key for the catalysts containing all PdOx substituted in the ceria lattice. On the other hand, catalysts containing both large surface supported PdO that is transformable to PdHx (in situ during the methane combustion reaction) and substituted PdOx were found to provide superior catalytic performance (complete CH4 conversion with 100% selectivity to CO2) with long life under dry and wet conditions. The discussed bifunctionality of the catalyst resulted in achieving a high TOF, high conversion and stability at elevated temperatures. Therefore, this study introduces a new strategy to improve the activity of combustion catalysts." @default.
- W3025232304 created "2020-05-21" @default.
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- W3025232304 date "2020-10-01" @default.
- W3025232304 modified "2023-09-26" @default.
- W3025232304 title "Engineering of catalytic sites of Pdx-Ce1-xO2-δ for dehydrogenation, oxygen insertion and reverse water gas shift reactions during methane combustion" @default.
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- W3025232304 doi "https://doi.org/10.1016/j.apcatb.2020.119118" @default.
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