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- W3025280451 endingPage "120089" @default.
- W3025280451 startingPage "120089" @default.
- W3025280451 abstract "The effects of composition on the iron redox equilibria and structural changes in the CaOAl2O3FetO melts have been investigated at 1823 K. The ferric to ferrous (Fe3+/Fe2+) ratio increases with increasing basicity and total iron oxide content when the activity of CaO (aCaO) is greater than 0.3. However, the Fe3+/Fe2+ ratios decrease with increasing iron oxide content in the case of the existence of octahedrally coordinated Fe3+ ions in aCaO=0.2 composition range. From Raman spectroscopic analysis, it was observed that the addition of iron oxide (up to 10 wt% T.Fe) to calcium aluminate melts modifies the aluminate networks. Furthermore, the non-bridging oxygen per tetrahedron (NBO/T) ratio in the CaOAl2O3FetO melts increases with increasing content of iron oxide because the [FeO4]-tetrahedron ferrite networks substitutes for the [AlO4]-tetrahedron aluminate networks. The activation energy for the viscous flow of the CaOAl2O3FetO melts has a good linear relationship with the relative concentration of polymerized [AlO4] unit, i.e., lnQAl4." @default.
- W3025280451 created "2020-05-21" @default.
- W3025280451 creator A5063292557 @default.
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- W3025280451 date "2020-08-01" @default.
- W3025280451 modified "2023-09-30" @default.
- W3025280451 title "Thermodynamics of iron redox equilibria and viscosity-structure relationship of CaO Al2O3FetO melts" @default.
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- W3025280451 doi "https://doi.org/10.1016/j.jnoncrysol.2020.120089" @default.
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