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- W3025385607 abstract "Severe deviation in structure and chemistry at grain boundaries has been regarded as the source of the poor conductivity of Li3xLa2/3-xTiO3. In this work, we report an in situ grain boundary engineering method to address this bottleneck. A lithium-rich electrolyte, Li3OCl, was introduced into Li3xLa2/3-xTiO3 to replenish lithium at the grain boundaries. Both the Li-gain on the boundary and generation of a Li-rich grain-engineered layer contributed to an optimized grain boundary conductivity of 1.52 × 10−4 (S/cm) and a depressed activation energy of 0.32 eV for grain boundary. Full batteries were further employed to demonstrate the enhancement in conductivity." @default.
- W3025385607 created "2020-05-21" @default.
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- W3025385607 date "2020-08-01" @default.
- W3025385607 modified "2023-10-14" @default.
- W3025385607 title "In situ atomic-scale engineering of the chemistry and structure of the grain boundaries region of Li3La2/3-TiO3" @default.
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- W3025385607 doi "https://doi.org/10.1016/j.scriptamat.2020.04.018" @default.
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