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• W3025632135 startingPage "122822" @default.
• W3025632135 abstract "Recently, photocatalytic NOx treatment has attracted great attention on account of the use of environmental-friendly and tremendous energy source. However, the difficult recovery of most reported powdery photocatalysts and the high generation rate of toxic NO2 byproduct limit its application. Here, we designed a novel monolithic protonated g-C3N4/graphene oxide aerogel through a direct frozen-drying method. A remarkable surface electric charge change of negative g-C3N4 to positive protonated g-C3N4 can be observed after the protonating treatment, which connects with negative graphene oxide nanosheets through the formation of strong electrostatic self-assembly to accelerate the photogenerated charge carriers transfer. Graphene oxide aerogel acts as a monolithic substrate, which provides abundant porous structure, enhanced visible-light absorption, and electrons transport pathway to improve photocatalytic activity. Importantly, the introduction of H atoms on the N atoms of p-C3N4 promotes the activation of oxygen atoms, thus improving the oxidization of NO2 to nitrate. As a result, protonated g-C3N4/graphene oxide aerogel reveals an excellent NO removal ratio (46.1%) and low NO2 generation (2.4%), demonstrating its excellent promising for air pollution purification. Our current work affords novel innovative insight for the construction of monolithic photocatalysts to control the secondary pollution for environmental remediation." @default.
• W3025632135 created "2020-05-21" @default.
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• W3025632135 date "2020-10-01" @default.
• W3025632135 modified "2023-10-13" @default.
• W3025632135 title "Surface modification to control the secondary pollution of photocatalytic nitric oxide removal over monolithic protonated g-C3N4/graphene oxide aerogel" @default.
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• W3025632135 doi "https://doi.org/10.1016/j.jhazmat.2020.122822" @default.
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