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• W3025687058 abstract "A new flexible cationic Zn(II)metal organic framework, {[Zn 2 (BDC) 1.5 (L)(DMF)]NO 3 · DMF·solvent } n , MOF 1 , which is a corrugated two‐dimensional network, was synthesized by self‐assembly of Zn(NO 3 ) 2 .6H 2 O with 4,4′‐methylenebis( N ‐(pyridin‐2‐ylmethylene)aniline as a neutral ligand and terephthalic acid in dimethyl formamide (DMF) as solvent and characterized by X‐ray diffraction. Because of the presence of uncoordinated nitrate (NO 3 − ) ions in the channels, the compound was employed for ion‐exchange applications. We report a detailed study of the host–guest interaction for a cationic metal–organic framework (MOF) that can reversibly capture nitrate. The recrystallization of the MOF was evaluated by monitoring the anion exchange dynamics using a combination of powder X‐ray diffraction and Fourier transform infrared spectra with various kinds of foreign anions. This MOF showed fast and highly efficient Cr 2 O 7 2− and CrO 4 2− , N 3 − , MnO 4 − , and SCN − exchange. The trapping capacities of Cr 2 O 7 2− , CrO 4 2− , N 3 − , MnO 4 − , and SCN − were 105,138, 44,104, and 25mg/g at 25°C after 3h, respectively, and there was good recyclability for capturing N 3 − and SCN − . {[Zn 2 (BDC) 1.5 (L)(DMF)]NO 3 } n exhibited anion exchange selectivity of SCN − in a solution containing a mixture of 0.025mmol N 3 − , SCN − , CrO 4 −2− , Cr 2 O 7 2− , and MnO 4 − for 3h and exhibited anion exchange selectivity for SCN − and Cr 2 O 7 2− in a solution containing a mixture of 0.001mmol N 3 − , SCN − , CrO 4 2− , Cr 2 O 7 2− , and MnO 4 − ." @default.
• W3025687058 created "2020-05-21" @default.
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• W3025687058 date "2020-05-15" @default.
• W3025687058 modified "2023-09-27" @default.
• W3025687058 title "2D → 3D corrugated structure self‐assembled from 4,4′‐methylenebis( <i>N</i> ‐(pyridin‐2‐ylmethylene)aniline and terephthalic acid: Crystal structure and selective anion separations via anion exchange" @default.
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• W3025687058 doi "https://doi.org/10.1002/aoc.5768" @default.
• W3025687058 hasPublicationYear "2020" @default.
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