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- W3025713025 endingPage "115785" @default.
- W3025713025 startingPage "115785" @default.
- W3025713025 abstract "Cu-based catalysts can experimentally catalyze the conversion of syngas-to-C2 oxygenates, however, since the chemical state of Cu sites dynamically evolves in the reaction process, no consensus has been reached on the precise roles of active Cuδ+(0 ≤ δ ≤ 1) sites. Here we resolve this long-term dispute with a series of highly comparable Cu catalyst. The results for the first time quantitatively identify the precise role of Cuδ(0 ≤ δ ≤ 1) sites in adjusting the catalytic activity and selectivity of syngas conversion over Cu-based catalysts, which is well illustrated in the view of electronic properties. Our quantitative results show that the moderate valence state Cuδ+(δ = 0.43 and 0.51) sites can highly-active and highly-selective catalyze the conversion of syngas to produce C2 oxygenates, which is also indirectly supported by the reported experiment studies. It is proposed that the balancing effect of Cu0 and Cu+ species in the experiment contribute to high catalytic performance toward the formation of C2 oxygenates." @default.
- W3025713025 created "2020-05-21" @default.
- W3025713025 creator A5000912155 @default.
- W3025713025 creator A5039456852 @default.
- W3025713025 creator A5042767652 @default.
- W3025713025 creator A5055496852 @default.
- W3025713025 creator A5062755510 @default.
- W3025713025 creator A5085814944 @default.
- W3025713025 date "2020-10-01" @default.
- W3025713025 modified "2023-10-14" @default.
- W3025713025 title "Syngas-to-C2 oxygenates on Cu-based catalyst: Quantitative insight into the balancing effect of active Cuδ+(0 ≤ δ ≤ 1) sites" @default.
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