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- W3025972357 abstract "Abstract Electrochemical behaviors of niobium sulfides such as 3 R -Nb 1+ x S 2 ( x = 0.00 ≈ 0.25), 2H-NbS 2 and NbS 3 for lithium batteries are investigated in 1 M LiClO 4 -propylene carbonate solution. The cathodic reaction in the charge-discharge cycle of the disulfides is shown as follows: X-ray diffraction measurement and open circuit potential data show that 3 R -Nb 1.00 S 2 gives continuous structural change along c-axis reversibly with cycling, where x takes from 0 to 1, whereas 2H-NbS 2 gives the stepwise change also reversibly with cycling, where x is at least 1. On the other hand, NbS 3 yields the ternary phase of Li x NbS 3 giving an amorphous X-ray pattern and shows irreversible structural change with cycling. When the charge-discharge cyclings are carried out at a constant capacity of 0.50 equivalent mole −1 of sulfide and a current density of 0.20 mA cm −2 , 3 R -Nb 1.00 S 2 can be cycled over 100 times without an increase in the charge potential, whereas in 2H-NbS 2 and NbS 3 the charge potentials rise to 4.6 V vs Li/Li + with cycling, which limits the cycle number to 30 ≈ 50 times. This would be due to the fact that 3 R -Nb 1.00 S 2 shows the reversible structural change with keeping the original crystal lattice with cycling." @default.
- W3025972357 created "2020-05-21" @default.
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- W3025972357 date "1982-11-23" @default.
- W3025972357 modified "2023-09-26" @default.
- W3025972357 title "ChemInform Abstract: CHARGE-DISCHARGE CHARACTERISTICS AND STRUCTURAL CHANGE IN VARIOUS NIOBIUM SULFIDE CATHODES FOR LITHIUM-NONAQUEOUS SECONDARY BATTERIES" @default.
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- W3025972357 doi "https://doi.org/10.1002/chin.198247020" @default.
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