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- W3027690752 abstract "A Mn-catalyzed diastereo- and enantioselective hydrogenation of α-substituted β-ketoamides has been realized for the first time under dynamic kinetic resolution conditions. anti-α-Substituted β-hydroxy amides, which are useful building blocks for the synthesis of bioactive molecules and chiral drugs, were prepared in high yields with excellent selectivity (up to >99 % dr and >99 % ee) and unprecedentedly high activity (TON up to 10000). The origin of the excellent stereoselectivity was clarified by DFT calculations." @default.
- W3027690752 created "2020-05-29" @default.
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- W3027690752 date "2020-07-01" @default.
- W3027690752 modified "2023-09-29" @default.
- W3027690752 title "Manganese‐Catalyzed <i>anti</i> ‐Selective Asymmetric Hydrogenation of α‐Substituted β‐Ketoamides" @default.
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- W3027690752 doi "https://doi.org/10.1002/anie.202006383" @default.
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