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- W3027977124 abstract "Abstract Buckyballs (fullerenes) were first reported over 30 years ago, but still little is known regarding their natural occurrence, since they have so far only been found at sites of high‐energy incidents, such as lightning strikes or meteor impacts, but have not been reported in low‐energy materials like fossil fuels. Using ultrahigh‐resolution mass spectrometry, a wide range of fullerenes from C 30 to C 114 was detected in the asphaltene fraction of a heavy crude oil, together with their building blocks of C 10n H 10 stoichiometry. High‐level DLPNO‐CCSD(T) calculations corroborate their stability as spherical and hemispherical species. Interestingly, the maximum intensity of the fullerenes was found at C 40 instead of the major fullerene C 60 . Hence, experimental evidence supported by calculations show the existence of not only buckyballs but also buckybowls as 3‐dimensional polyaromatic compounds in fossil materials." @default.
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- W3027977124 date "2020-06-17" @default.
- W3027977124 modified "2023-10-03" @default.
- W3027977124 title "Studying Natural Buckyballs and Buckybowls in Fossil Materials" @default.
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- W3027977124 doi "https://doi.org/10.1002/anie.202005449" @default.
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