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• W3029103958 abstract "The development of new amide precursors for selective, catalytic activation of carbon-nitrogen bonds in amides is a fundamental objective of this emerging reactivity manifold. We report the palladium-catalyzed Suzuki-Miyaura cross-coupling of N-acylcarbazoles and N-acylindoles with arylboronic acids by a highly selective N-C(O) cleavage. The key amide bond ground-state destabilization stems from Nlp to Ar conjugation and enables us for the first time to achieve reactivity similar to that for N-acylsulfonamide and N-acylcarbamate activation in simple anilides." @default.
• W3029103958 created "2020-06-05" @default.
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• W3029103958 date "2020-06-01" @default.
• W3029103958 modified "2023-10-14" @default.
• W3029103958 title "<i>N</i>-Acylcarbazoles and <i>N</i>-Acylindoles: Electronically Activated Amides for N–C(O) Cross-Coupling by N_lp to Ar Conjugation Switch" @default.
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• W3029103958 doi "https://doi.org/10.1021/acs.orglett.0c01488" @default.
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• W3029103958 hasPublicationYear "2020" @default.
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