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- W3033146103 abstract "High-energy strained liquid fuels are critical to improving the payload and flight distance of advanced propulsion. This chapter will summarize the synthesis and properties of high-energy strained liquid fuels including quadricyclane, cyclopropane fuel, spiro-fuel, and other caged fuels. Firstly, photocatalytic synthesis of quadricyclane with high volumetric heat value and high density is introduced, which mainly includes homogeneous reaction mechanism and heterogeneous photocatalysis reaction mechanism and the involved catalysts. Later, the cyclopropanation reaction to synthesize the cyclopropane-based fuel with high calorific value and high tension is summarized, mainly including two kinds of reactions: organometallic carbenoid reagent-mediated cyclopropanation and transition metal carbene-mediated cyclopropanation. In addition, the mechanism of cyclopropanation was presented by taking endo-dicyclopentadiene and zinc carbenoid as examples. Finally, the synthesis and properties of some spiro-fuels, PCU-derived fuels, cubane-based fuels, and other caged fuels are comprehensively reviewed. This chapter will be helpful to explore better strategy for the synthesis of high-energy strained fuels for advanced propulsion applications." @default.
- W3033146103 created "2020-06-12" @default.
- W3033146103 creator A5001687232 @default.
- W3033146103 creator A5038458746 @default.
- W3033146103 creator A5041668330 @default.
- W3033146103 creator A5091499047 @default.
- W3033146103 date "2020-06-05" @default.
- W3033146103 modified "2023-10-03" @default.
- W3033146103 title "Design and Synthesis of High‐Energy Strained Fuels" @default.
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