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- W3033271225 abstract "This is a new fundamental theory of the interfacial energy including the explicit formulation of interfacial energy in a single formula, which involves the essential concept of the interfacial energy and all elements of the Gibbs, Langmuir, and Szyszkowski adsorption equations. The present thermodynamic theory is based on deductive conclusions that the intrinsic interfacial chemical potential of each component is generally higher than the bulk one at equilibrium and that the source of the interfacial energy is the excess chemical potential of each interfacial component. In addition, from an insight into the nature of interfaces, an interfacial double layer model has been proposed. The derived fundamental equation of the specific interfacial energy (γ) at equilibrium is given as γ =Nσi([formula]− μαi) +Nσj([formula]− μβj), whereNσiandNσjare the two-dimensional maximum molar densities of arbitrary componentsiandjin the surface layers of a limited thickness, σAand σB, of two adjoining bulk phases α and β, respectively; μiand μjare the chemical potentials of componentsiandjin the phases indicated by the superscripts. Hence, γ consists of the specific surface energies of the σA- and σB-layers, γA(=Nσi([formula]− μαi) =NσA([formula]− μαA)) and γB(=Nσj([formula]− μβj) =NσB([formula]− μβB)), respectively, whereAandBare the matrix components of the α- and β-phases, respectively." @default.
- W3033271225 created "2020-06-12" @default.
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- W3033271225 date "1996-07-01" @default.
- W3033271225 modified "2023-09-25" @default.
- W3033271225 title "A New Approach to Interfacial Energy" @default.
- W3033271225 doi "https://doi.org/10.1006/jcis.1996.0377" @default.
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