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- W3033632022 endingPage "122458" @default.
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- W3033632022 abstract "Abstract In order to alleviate the corrosion of metal in the pickling process, three kinds of N-doped carbon dots (N-CDs) inhibitors were obtained via the decomposition of natural citric acid derivative under various preparation temperatures (150, 180, 210 °C) for 2 h. Structural characterizations showed that N element was successfully doped into the carbon dots to form pyridine-like N, pyrrole-like N and graphitic N. Electrochemistry results implied that the corrosion current density of steel in 200 mg/L of N-CDs solutions was 24.1, 10.7 and 40.4 μA/cm2, which was greatly lower than that in 1 M HCl environment. In this case, the inhibitive efficiency of these N-CDs was higher than 90%. Through calculation, the standard adsorption free energy (ΔG0ads) of as-prepared N-CDs was −25.99, −26.94 and −25.78 kJ/mol, indicating that the adsorption film involved both physisorption and chemisorption. Furthermore, the molecular simulation calculation suggested that the as-prepared N-CDs were parallelly adsorbed on the steel/solution interface. This novel and green corrosion inhibitor was promising to solve the corrosion problem of metal equipment in the acidic process." @default.
- W3033632022 created "2020-06-12" @default.
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- W3033632022 date "2020-10-01" @default.
- W3033632022 modified "2023-10-03" @default.
- W3033632022 title "Corrosion inhibition behavior and mechanism of N-doped carbon dots for metal in acid environment" @default.
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- W3033632022 doi "https://doi.org/10.1016/j.jclepro.2020.122458" @default.
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