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- W3033879428 abstract "In this study, we present the synthesis and full characterization of the dimer Ni(II) complex, [Ni2(dpaa)2(bpy)2(SO4)(H2O)]CH3OH, (dpaa = diphenyl acetic acid, bpy = 2,2′-bipyridine) with an N2O4 donor set and its hydrogenation activity on linear and cyclic alkenes (1-octene, t-2-octene, 1-hexene, cyclohexene, cyclopentene, benzene and styrene) with NaBH4 as a hydrogen source. 1-Octene and 1-hexene were reduced to the corresponding alkanes as the major products (81.3 and 91.2%, respectively), and the substrate isomerized the terminal alkenes to a mixture of internal alkenes as minor products (1–4%) under the studied conditions (subs/cat/reduct. 100/1/1 in methanol, 40 °C, 6 h). To optimize the reaction conditions for the reduction of styrene to ethyl benzene in methanol, the effect of subs./NaBH4 ratio, solvent and temperature were also investigated." @default.
- W3033879428 created "2020-06-12" @default.
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- W3033879428 date "2020-09-01" @default.
- W3033879428 modified "2023-09-27" @default.
- W3033879428 title "Bimetallic Ni(II) complex with carboxylate bridging for homogeneous hydrogenation of alkenes with NaBH4" @default.
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- W3033879428 doi "https://doi.org/10.1016/j.poly.2020.114649" @default.
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