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- W3034503160 abstract "The (Mn,Fe)2(P,Si) compounds with large magnetocaloric effect are sensitive to the contents of impurity phase. In order to decrease its contents, the (MnFe)δ(P0.5Si0.5) (δ = 1.90, 1.95, 2.00, 2.05) compounds were designed and prepared by arc-melting method. The structure and magnetic properties were characterized by XRD, SEM, DSC and VSM, respectively. The diffraction analysis reveals that all samples are hexagonal Fe2P-type crystals with some impurity phase. The structure of impurity phase would change from cubic (Mn,Fe)3Si to hexagonal (Mn,Fe)5Si3 with decreasing δ from 2.05 to 1.90. And the Curie temperature of (MnFe)δ(P0.5Si0.5) compounds increased from 234 K for δ = 2.05 to 371 K for δ = 1.90. Meanwhile, the thermal hysteresis decreased by 58%. Under the field change of 5 T, the peak values of isothermal entropy change reaches 19.6 J‧kg−1‧K−1 for δ = 1.95. While, the maximal adiabatic temperature change increased by 47% as δ decreasing from 2.05 to 1.90. All results show that the impurity phase and magnetic properties of the (Mn,Fe)2(P,Si) compounds can be effectively tuned by adjusting M/NM ratios." @default.
- W3034503160 created "2020-06-19" @default.
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- W3034503160 date "2020-10-01" @default.
- W3034503160 modified "2023-10-12" @default.
- W3034503160 title "Effect of M/NM ratios on structural and magnetic properties of (Mn,Fe)2(P,Si) compounds" @default.
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- W3034503160 doi "https://doi.org/10.1016/j.physb.2020.412309" @default.
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