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• W3035089860 abstract "This study compared the hydrodeoxygenation (HDO) of m-cresol over Pt and NbOx-modified Pt catalysts. Reactivity measurements demonstrated that Pt supported on carbon (Pt/C) has moderate selectivity for the production of toluene during the HDO of m-cresol, with a range of ring saturation products also being produced. The modification of Pt with niobium (NbOx–Pt/C), however, was found to enhance the selectivity to toluene to 95%. Temperature-programmed desorption, X-ray photoelectron spectroscopy, and high-resolution electron energy loss spectroscopy studies of model Pt(111) single crystal catalysts were used to provide insight into the mechanism by which the niobium enhances the selectivity. These studies showed that interactions at the NbOx–Pt interface help maintain the niobium in a partially reduced state that contains unsaturated Nb cations, which provide adsorption sites on which m-cresol undergoes direct C–O bond hydrogenolysis to produce toluene." @default.
• W3035089860 created "2020-06-19" @default.
• W3035089860 creator A5010837144 @default.
• W3035089860 creator A5052988578 @default.
• W3035089860 date "2020-06-08" @default.
• W3035089860 modified "2023-10-18" @default.
• W3035089860 title "Direct Hydrodeoxygenation of <i>m</i>-Cresol to Toluene over Bifunctional NbO_<i>x</i>–Pt" @default.
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• W3035089860 doi "https://doi.org/10.1021/acs.jpcc.0c03988" @default.
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