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- W3036170141 abstract "In this work, an ultrafast spectral diffusion of the lowest exciton in a tetracene ultrathin film is studied by two-dimensional electronic spectroscopy. From the analysis of the nodal line slope, the frequency-fluctuation correlation function (FFCF) of the exciton band is extracted. The FFCF contains two components with decay times of 400 and 80 fs; while the former can be understood by a linear exciton–phonon coupling model, the latter shows an order of magnitude increase in its amplitude from 96 to 186 K that cannot be explained by the same model. A novel scheme of the energy-gap fluctuations is examined, in which an intramolecular high-frequency mode causes the spectral diffusion that is enhanced through an anharmonic coupling to low-frequency phonon modes. This finding provides a valuable input for future theoretical predictions on the ultrafast nonadiabatic dynamics of the molecular exciton." @default.
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- W3036170141 date "2020-06-18" @default.
- W3036170141 modified "2023-09-27" @default.
- W3036170141 title "Anomalous Temperature Dependence of Exciton Spectral Diffusion in Tetracene Thin Film" @default.
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- W3036170141 doi "https://doi.org/10.1021/acs.jpclett.0c01537" @default.
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