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- W3036405330 abstract "Abstract Hyperbranched polymers have garnered much attention due to attractive properties and wide applications, such as drug‐controlled release, stimuli‐responsive nano‐objects, photosensitive materials and catalysts. Herein, two types of novel hyperbranched poly(ester‐enamine) (hb‐PEEa) were designed and synthesized via the spontaneous amino‐yne click reaction of A 2 monomer (1, 3‐bis(4‐piperidyl)‐propane (A 2a ) or piperazine (A 2b )) and B 3 monomer (trimethylolpropanetripropiolate). According to Flory's hypothesis, gelation is an intrinsic problem in an ideal A 2 +B 3 polymerization system. By controlling the polymerization conditions, such as monomer concentration, molar ratio and rate of addition, a non‐ideal A 2 +B 3 polymerization system can be established to avoid gelation and to synthesize soluble hb‐PEEa. Due to abundant unreacted alkynyl groups in periphery, the hb‐PEEa can be further functionalized by different amino compounds or their derivates. The as‐prepared amphiphilic PEG‐hb‐PEEa copolymer can readily self‐assemble into micelles in water, which can be used as surfactant to stabilize Au nanoparticles (AuNPs) during reduction of NaBH 4 in aqueous solution. As a demonstration, the as‐prepared PEG‐hb‐PEEa‐supported AuNPs demonstrate good dispersion in water, solvent stability and remarkable catalytic activity for reduction of nitrobenzene compounds." @default.
- W3036405330 created "2020-06-25" @default.
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- W3036405330 date "2020-07-06" @default.
- W3036405330 modified "2023-10-06" @default.
- W3036405330 title "Hyperbranched Poly(ester‐enamine) from Spontaneous Amino‐yne Click Reaction for Stabilization of Gold Nanoparticle Catalysts" @default.
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- W3036405330 doi "https://doi.org/10.1002/asia.202000621" @default.
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