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• W3036773922 endingPage "127427" @default.
• W3036773922 startingPage "127427" @default.
• W3036773922 abstract "Spinel oxides, e.g., NiCo2O4, is a promising catalyst for the catalytic oxidation of toluene. Understanding and designing versatile NiCo2O4 spinel is important for low-temperature toluene oxidation. Here, we investigated the surface-characteristic-dependent degradation activity of NiCo2O4 crystals through experiment and characterization. NiCo2O4 nanosheet using ethanol as solvent (named E--NiCo2O4) exposing {110} crystal planes exhibited the lowest temperature toluene oxidation. The T99 of toluene conversion was 256 °C, which is much lower than that of NiCo2O4 nanosheet using ethylene glycol as solvent (named EG--NiCo2O4), NiCo2O4 octahedron (named O--NiCo2O4) and NiCo2O4 truncated octahedron (named TO--NiCo2O4). Characterization using various techniques such as XRD, TEM, BET, XPS, H2-TPR and CO2-TPD showed that Co3+ and surface adsorbed oxygen (Osur) enriched surface, excellent redox properties and effective diffusion of the reaction product reasonably explain the enhancement in catalytic activity over the E--NiCo2O4. The research reveals that the effect of specific crystal planes and solvent was the key factor to govern the activity of low-temperature toluene oxidation." @default.
• W3036773922 created "2020-06-25" @default.
• W3036773922 creator A5032694602 @default.
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• W3036773922 date "2020-11-01" @default.
• W3036773922 modified "2023-10-11" @default.
• W3036773922 title "NiCo2O4 spinel for efficient toluene oxidation: The effect of crystal plane and solvent" @default.
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• W3036773922 doi "https://doi.org/10.1016/j.chemosphere.2020.127427" @default.
• W3036773922 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32599385" @default.
• W3036773922 hasPublicationYear "2020" @default.
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