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- W3036883941 endingPage "5745" @default.
- W3036883941 startingPage "5741" @default.
- W3036883941 abstract "Herein, we show that biradical character and appropriate distribution of spin density can be used for synthetic purposes. We demonstrate the rational domino annulation that includes dehydrative π-extension (DPEX) as the initiation step and subsequent oxidative electrocyclizations (EC) promoted by favorable localization of the unpaired electrons enabling up to four C–C bonds formed during the reaction. Contradicting to the Woodward–Hoffmann rules, the reaction proceeds at room temperature, whereas termination occurs when biradical character vanishes." @default.
- W3036883941 created "2020-06-25" @default.
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- W3036883941 date "2020-06-17" @default.
- W3036883941 modified "2023-09-28" @default.
- W3036883941 title "Oxidative Electrocyclization of Diradicaloids: C–C Bonds for Free or How to Use Biradical Character for π-Extension" @default.
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- W3036883941 doi "https://doi.org/10.1021/acs.orglett.0c01717" @default.
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