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• W3036952033 abstract "Abstract Product selectivity control is attractive in Fischer-Tropsch (F-T) synthesis but it is still a challenge, because the F-T products follow the Anderson-Schulz-Flory (ASF) distribution with maximized gasoline-ranged (C5−C11) hydrocarbon selectivity at 45%. Herein, we report a strategy by optimizing the gasoline selectivity to outperform the ASF limitation. The key to this success is fixation of the metal nanoparticles within zeolite crystals (metal@zeolite), where the zeolite micropore adjusts the product selectivity. For example, the Ru@NaY exhibited the gasoline selectivity 64.3% in the F-T reaction, which is significantly higher than the ASF limitation and about 2 times of that (32.8%) over conventionally supported Ru catalyst (Ru/NaY). This investigation might offer an alternative route for the direct transformation of syngas to liquid fuels with controllable selectivities." @default.
• W3036952033 created "2020-06-25" @default.
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• W3036952033 date "2021-03-01" @default.
• W3036952033 modified "2023-10-14" @default.
• W3036952033 title "Fischer-Tropsch reaction within zeolite crystals for selective formation of gasoline-ranged hydrocarbons" @default.
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• W3036952033 doi "https://doi.org/10.1016/j.jechem.2020.06.006" @default.
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