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• W3037071575 endingPage "118494" @default.
• W3037071575 startingPage "118494" @default.
• W3037071575 abstract "Pyrolytic char is widely used for tar removal due to its cost-effective and eco-friendly. In this work, the waste municipal sludge is selected to produce the composite catalyst with transition metal Fe/Ni, and the as-synthesized catalyst was used in the catalytic cracking of the tar model compound toluene by a laboratory-scale plant. The toluene conversion and the molar ratios of CO, H2, CO2, CH4 and C2H4 in the generated gas were investigated. Results show that municipal sludge char-based catalysts are more likely to produce H2-rich syngas (the molar ratio of syngas > 75%), and the molar ratio of H2 can reach 73.3% under optimal conditions. The Fe-Ni bimetallic catalyst combines the advantages of different metal elements to make the catalyst performance more stable. Meanwhile, the effects of residence time (τ) and steam-to-carbon ratio (S/C) on the conversion rate were studied. As a result, the excessive residence time or steam-to-carbon ratio will have no more positive effect on the performance of the catalyst. Ultimately, the catalyst life test of 8 h was carried out, the results showed that cost-effective and green waste municipal sludge char-supported Fe/Ni catalysts in this work could be used for removal of the tar heavy component toluene." @default.
• W3037071575 created "2020-07-02" @default.
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• W3037071575 date "2020-11-01" @default.
• W3037071575 modified "2023-09-23" @default.
• W3037071575 title "Pyrolysis municipal sludge char supported Fe/Ni catalysts for catalytic reforming of tar model compound" @default.
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• W3037071575 doi "https://doi.org/10.1016/j.fuel.2020.118494" @default.
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