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• W3037202862 abstract "Assembling Ti3C2Tx MXene nanosheets into three-dimensional (3D) architecture with controllable alignment is of great importance for electromagnetic wave absorption (EMA) application. However, it is a great challenge to realize it due to the weak van der Waals interconnection between MXene nanosheets. Herein, we propose to introduce gelatin molecules as a chemical glue to fabricate the 3D Mxene@gelatin (M@G) nanocomposite aerogel using a unidirectional freeze casting method. The Ti3C2Tx MXene nanosheets are well aligned in the M@G nanocomposite aerogel, yielding much enhanced yet anisotropic mechanical properties. Due to the unidirectional aligned microstructure, the M@G nanocomposite aerogel shows significantly anisotropic EMA properties. M@G-45 shows a -59.5 dB minimum reflection loss (RLmin) at 14.04 GHz together with a 6.24 GHz effective absorption bandwidth in the parallel direction (relative to the direction of unidirectional freeze casting). However, in the vertical direction of the same M@G aerogel, RLmin is shifted to a much lower frequency (4.08 GHz) and the effective absorption bandwidth decreases to 0.86 GHz. The anisotropic electromagnetic energy dissipation mechanism was deeply investigated, and the impendence match plays a critical role for electromagnetic wave penetration. Our lightweight M@G nanocomposite aerogel with controllable MXene alignment is very promising in EMA application." @default.
• W3037202862 created "2020-07-02" @default.
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• W3037202862 date "2020-06-29" @default.
• W3037202862 modified "2023-10-16" @default.
• W3037202862 title "Anisotropic Electromagnetic Absorption of Aligned Ti₃C₂T<i>_x</i> MXene/Gelatin Nanocomposite Aerogels" @default.
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• W3037202862 doi "https://doi.org/10.1021/acsami.0c09726" @default.
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