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• W3037478997 abstract "Polymeric nitrogen at 120 GPa–180 GPa is known in two monatomic crystalline cubic gauche (cg-N) and layered polymeric (LP-N) phases and one amorphous modification (η-N), and all these high-pressure phases attract considerable attention for their potential application as a high energy density material. Here, we investigated the stability of these modifications at high pressures in the laser heated diamond anvil cell upon decompression from 161 GPa. Pure LP-N was synthesized above 152 GPa upon laser heating of η-N to 2500 K, while cg-N forms below 150 GPa. Upon laser heating at 129 GPa and 123 GPa, the LP-N clearly diminished, indicating that the synthesis of cg-N becomes more favorable in a mixed phase region below 129 GPa. Upon unloading, cg-N and LP-N were metastable to at least 71 GPa at up to 2500 K and at room temperature, respectively. These observations clarified a complicated polymorphism of monatomic nitrogen at high pressures and large hysteretic phenomena related to a transition to nonmolecular nitrogen." @default.
• W3037478997 created "2020-07-02" @default.
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• W3037478997 date "2020-06-25" @default.
• W3037478997 modified "2023-10-01" @default.
• W3037478997 title "Polymorphism of polymeric nitrogen at high pressures" @default.
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• W3037478997 doi "https://doi.org/10.1063/5.0007453" @default.
• W3037478997 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32610991" @default.
• W3037478997 hasPublicationYear "2020" @default.
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