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- W3037487544 abstract "Two new operation modes, “pink beam” excitation, which has the energy bandwidth defined by X-ray mirrors and filters, and “broadband beam”, where the energy bandwidth is defined by the reflection from a multilayer monochromator, were implemented at the SuperXAS beamline of the Swiss Light Source (SLS). These setups allow measuring non-resonance X-ray emission spectra (XES) with 2–3 orders of magnitude higher incident flux than non-resonant XES measurements with a monochromatic incident beam. For the broadband beam mode, a Mo/Si multilayer structure was designed, with which the energy can be tuned in the 5–17 keV range. The multilayer demonstrates a relatively large energy bandwidth of 4 ± 0.2% through the whole energy range and a reflectivity of 23–60%, which increases with energy. We show that by using pink beam mode one can investigate the electronic structure of photocatalytic intermediates through time-resolved core-to-core XES experiments of diluted samples with a concentration of the element of interest of ~1 mM. Broadband beam mode is optimal for valence-to-core XES experiments and allow to avoid the excitation of additional KLβ satellites that can complicate the interpretation of spectra." @default.
- W3037487544 created "2020-07-02" @default.
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- W3037487544 date "2020-09-01" @default.
- W3037487544 modified "2023-10-03" @default.
- W3037487544 title "Operation of a bending magnet beamline in large energy bandwidth mode for non-resonant X-ray emission spectroscopy" @default.
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- W3037487544 doi "https://doi.org/10.1016/j.rinp.2020.103212" @default.
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