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• W3038346319 endingPage "118449" @default.
• W3038346319 startingPage "118449" @default.
• W3038346319 abstract "Abstract Dual-layer slot coating (DSC) is a state-of-the-art technique that can fabricate thin film composite membranes by simultaneously spreading two monomer solutions to form an unsupported ultrathin polyamide (PA) selective layer, which is subsequently adhered to a support. To demonstrate its versatility, DSC was applied to polyethylene and polysulfone supports modified with O2 plasma and/or polydopamine (PDA) coating for the fabrication of high-performance reverse osmosis (RO) membranes. PDA coating enabled the uniform and robust PA deposition by uniformly hydrophilizing supports and reinforcing PA-support interfacial adhesion through the introduction of oxygen-containing and amine groups that promote hydrogen bonding with the PA layer, thus achieving good RO performance. The O2 plasma treatment on PDA-coated supports further strengthened PA-support interfacial adhesion by increasing the number of carboxyl groups with a higher hydrogen bonding ability, hence fabricating long-term stable, high-performance RO membranes that outperform a commercial RO membrane. This superior RO performance was enabled by the extremely thin (~7 nm) and highly crosslinked PA structure as well as strong PA-support interfacial adhesion. The surface tension analysis suggested that the work of adhesion at the PA-support interface of >~110 mJ m−2 is required to achieve high membrane performance." @default.
• W3038346319 created "2020-07-10" @default.
• W3038346319 creator A5059530002 @default.
• W3038346319 creator A5087337598 @default.
• W3038346319 date "2020-11-01" @default.
• W3038346319 modified "2023-10-17" @default.
• W3038346319 title "Fabrication of high-performance reverse osmosis membranes via dual-layer slot coating with tailoring interfacial adhesion" @default.
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• W3038346319 doi "https://doi.org/10.1016/j.memsci.2020.118449" @default.
• W3038346319 hasPublicationYear "2020" @default.
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