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• W3039587391 endingPage "095009" @default.
• W3039587391 startingPage "095009" @default.
• W3039587391 abstract "Abstract Plasma has been studied for several years to convert CO 2 into value-added products. If CO 2 could be converted in the presence of H 2 O as a cheap H-source for making syngas and oxygenates, it would mimic natural photosynthesis. However, CO 2 /H 2 O plasmas have not yet been extensively studied, not by experiments, and certainly not computationally. Therefore, we present here a kinetic modelling study to obtain a greater understanding of the vibrational kinetics of a CO 2 /H 2 O microwave plasma. For this purpose, we first created an electron impact cross section set for H 2 O, using a swarm-derived method. We added the new cross section set and CO 2 /H 2 O-related chemistry to a pure CO 2 model. While it was expected that H 2 O addition mainly causes quenching of the CO 2 asymmetric mode vibrational levels due to the additional CO 2 /H 2 O vibrational-translational relaxation, our model shows that the modifications in the vibrational kinetics are mainly induced by the strong electron dissociative attachment to H 2 O molecules, causing a reduction in electron density, and the corresponding changes in the input of energy into the CO 2 vibrational levels by electron impact processes." @default.
• W3039587391 created "2020-07-10" @default.
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• W3039587391 date "2020-09-01" @default.
• W3039587391 modified "2023-10-18" @default.
• W3039587391 title "The effect of H₂O on the vibrational populations of CO₂ in a CO₂/H₂O microwave plasma: a kinetic modelling investigation" @default.
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• W3039587391 doi "https://doi.org/10.1088/1361-6595/aba1c8" @default.
• W3039587391 hasPublicationYear "2020" @default.
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