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- W3039709145 abstract "Abstract We disclose a new Brønsted acid promoted quinoline synthesis, proceeding via homo‐diaza‐Cope rearrangement of N ‐aryl‐ N ′‐cyclopropyl hydrazines. Our strategy can be considered a homologation of Fischer's classical indole synthesis and delivers 6‐membered N‐heterocycles, including previously inaccessible pyridine derivatives. This approach can also be used as a pyridannulation methodology toward constructing polycyclic polyheteroaromatics. A computational analysis has been employed to probe plausible activation modes and to interrogate the role of the catalyst." @default.
- W3039709145 created "2020-07-10" @default.
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- W3039709145 date "2020-09-07" @default.
- W3039709145 modified "2023-10-18" @default.
- W3039709145 title "Homologation of the Fischer Indolization: A Quinoline Synthesis via Homo‐Diaza‐Cope Rearrangement" @default.
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- W3039709145 doi "https://doi.org/10.1002/anie.202005798" @default.
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