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- W3040111237 endingPage "12607" @default.
- W3040111237 startingPage "12602" @default.
- W3040111237 abstract "The first and asymmetric total synthesis of bioactive bufospirostenin A, an unusual spirostanol with rearranged A/B rings, was accomplished. The synthetically challenging [5–7–6–5] tetracyclic ring system, found in bufospirostenin A and some other natural products, was efficiently constructed by the unique intramolecular rhodium-catalyzed Pauson–Khand reaction of an alkoxyallene-yne. The 11 stereocenters in the final product, including the 10 contiguous stereocenters, were installed diastereoselectively." @default.
- W3040111237 created "2020-07-10" @default.
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- W3040111237 date "2020-07-06" @default.
- W3040111237 modified "2023-10-17" @default.
- W3040111237 title "Asymmetric Total Synthesis of Bufospirostenin A" @default.
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- W3040111237 doi "https://doi.org/10.1021/jacs.0c05479" @default.
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