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• W3040366387 endingPage "109597" @default.
• W3040366387 startingPage "109597" @default.
• W3040366387 abstract "An accurate knowledge of the electrical properties of molten salts and slags is important for the design, optimization and control of several electrochemical processes. The electrical conductivity of molten salts and slags is in principle of ionic nature, however when metals are dissolved in electrolyte electrons may also contribute to the electrical conductivity. Only a few studies reporting an electronic conductivity of simple molten salts can be found in the literature and the microscopic aspect of the electron transport within ionically bonded systems remains vague. The aim of this work is to fill-up this gap. To do so, a new theoretical model, based on the Boltzmann transport equation, is developed to represent the electronic conductivity of metals diluted in molten salt systems at up to about 10 mol% of metal. It is shown that the proposed model has a good predictive capability for most molten salts-metal systems for which experimental data is available. Then, based on this approach, the electronic conductivity of different cryolitic melts of interest for the aluminum production industry are predicted. Particular attention is drawn to the melts containing both lithium and potassium fluorides as they are considered as potential additives for the next reduction cells generation. A good agreement is obtained with the only available set of experimental data for standard electrolytes reported by Haarberg et al. (1996), indicating on one hand the predictive capability of the model for more complex systems (i.e. those with a significant short range ordering) and on the other hand the reliability of our predictions for all cryolitic melts as a function of the cryolitic ratio, temperature and additive amount." @default.
• W3040366387 created "2020-07-10" @default.
• W3040366387 creator A5051617334 @default.
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• W3040366387 date "2020-09-01" @default.
• W3040366387 modified "2023-10-17" @default.
• W3040366387 title "Modelling the electronic conduction in metals-molten salts mixtures. Application to cryolitic melts in Hall-Héroult cells" @default.
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• W3040366387 doi "https://doi.org/10.1016/j.jfluchem.2020.109597" @default.
• W3040366387 hasPublicationYear "2020" @default.
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