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- W3040398613 abstract "Abstract Electrochemical oxidation (EO) is a promising technique for decentralized wastewater treatment, owing to its modular design, high efficiency, and ease of automation and transportation. The catalytic destruction of recalcitrant, non-biodegradable pollutants (per- and poly-fluoroalkyl substances (PFAS), pharmaceuticals, and personal care products (PPCPs), pesticides, etc.) is an appropriate niche for EO. EO can be more effective than homogeneous advanced oxidation processes for the degradation of recalcitrant chemicals inert to radical-mediated oxidation, because the potential of the anode can be made much higher than that of hydroxyl radicals (E OH = 2.7 V vs. NHE), forcing the direct transfer of electrons from pollutants to electrodes. Unfortunately, at such high anodic potential, chloride ions, which are ubiquitous in natural water systems, will be readily oxidized to chlorine and perchlorate. Perchlorate is a to-be-regulated byproduct, and chlorine can react with matrix organics to produce organic halogen compounds. In the past ten years, novel electrode materials and processes have been developed. However, spotlights were rarely focused on the control of byproduct formation during EO processes in a real-world context. When we use EO techniques to eliminate target contaminants with concentrations at µg/L-levels, byproducts at mg/L-levels might be produced. Is it a good trade-off? Is it possible to inhibit byproduct formation without compromising the performance of EO? In this minireview, we will summarize the recent advances and provide perspectives to address the above questions." @default.
- W3040398613 created "2020-07-10" @default.
- W3040398613 creator A5016521913 @default.
- W3040398613 date "2020-06-30" @default.
- W3040398613 modified "2023-10-14" @default.
- W3040398613 title "Recent advances in the electrochemical oxidation water treatment: Spotlight on byproduct control" @default.
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- W3040398613 doi "https://doi.org/10.1007/s11783-020-1264-7" @default.
- W3040398613 hasPublicationYear "2020" @default.
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