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• W3040805963 startingPage "6127" @default.
• W3040805963 abstract "Clusters consisting of 20 water molecules and a single cesium ion are especially stable due to their clathrate structure that is composed exclusively of three-coordinate water molecules. Clathrate stability was investigated using infrared photodissociation (IRPD) spectroscopy in the free-OH stretching region (∼3600–3800 cm–1) at ion cell temperatures between 135 and 355 K. At 275 K and colder, IRPD spectra of Cs+(H2O)20 have just one acceptor–acceptor–donor band. At higher temperatures, a higher-energy acceptor–donor band emerges and grows in intensity. Non-clathrate Na+(H2O)20 structures contain both of these bands, which do not change significantly in intensity over the temperature range. These results indicate a rapid onset in the conversion from clathrate to non-clathrate structures with temperature and suggest that some clathrate population remains even at the highest temperatures investigated. These results provide new insights into the role of entropy in clathrate stability." @default.
• W3040805963 created "2020-07-16" @default.
• W3040805963 creator A5014296444 @default.
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• W3040805963 date "2020-07-07" @default.
• W3040805963 modified "2023-09-25" @default.
• W3040805963 title "Effects of Temperature on Cs⁺(H₂O)₂₀ Clathrate Structure" @default.
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• W3040805963 doi "https://doi.org/10.1021/acs.jpclett.0c01554" @default.
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• W3040805963 hasPublicationYear "2020" @default.
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