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• W3041882592 endingPage "136746" @default.
• W3041882592 startingPage "136746" @default.
• W3041882592 abstract "• Construction of spiny PPy arrays on flexible textile electrode is successfully achieved. • The solid-state EPPy-PPy/NF/CF supercapacitor exhibits superior cycle stability. • The combined effect of micelles and bubbles on the formation of the spiny PPy are elucidated. • This supercapacitor demonstrates its great potential in wearable electronics. The most explored flexible supercapacitors based on PPy electrodes face a huge challenge of poor cycle performance. Here, we demonstrate successful construction of sea urchin spines-like PPy arrays on cotton-based fabric electrode via a facile electropolymerization and employ it in enhancing the cyclic stability of the supercapacitors without recombination of PPy with other capacitive materials. This novel fabric electrode (called EPPy-PPy/NF/CF) consists of a cotton fabric (CF) coated with PVA- co -PE nanofibers (NF) as a flexible substrate (NF/CF). The formation mechanism of the spiny PPy with nanocavities is explored, and the effects of surface wettability of the support electrode (PPy/NF/CF), micellar size, and bubble generation on the nucleation and growth of the PPy during electropolymerization are elucidated. Significantly, the flexible solid-state symmetrical EPPy-PPy/NF/CF supercapacitor exhibits striking cycling stability with 100% retention after 10,000 cycles at a current density of 4 mA cm −2 . The superior cyclic stability can be attributed to the spiny PPy arrays, which can shorten the transmission paths of counter ions and charges, thereby weakening stress-induced damages to the PPy skeleton. Additionally, this flexible supercapacitor also shows a great potential for application in portable and wearable electronic devices." @default.
• W3041882592 created "2020-07-16" @default.
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• W3041882592 date "2020-09-01" @default.
• W3041882592 modified "2023-10-16" @default.
• W3041882592 title "The construction of sea urchin spines-like polypyrrole arrays on cotton-based fabric electrode via a facile electropolymerization for high performance flexible solid-state supercapacitors" @default.
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• W3041882592 doi "https://doi.org/10.1016/j.electacta.2020.136746" @default.
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