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- W3042247998 abstract "Uniform lithium (Li) deposition in all-solid-state Li metal batteries is greatly influenced by the anode/electrolyte interface. Herein, a Mg-modified interface was constructed via the simple in-situ electrochemical reduction of Mg2+ from Mg(TFSI)2 in polyethylene oxide (PEO) and a Li bis(trifluoromethane)sulfonimide (LiTFSI) formulae. As confirmed by cryogenic transmission electron microscopy, the anode/electrolyte interface exhibited hybrids consisting of crystalline Mg, Li2O, and Li dots embedded in an amorphous polymer electrolyte. The crystalline Mg dots guided the uniform Li nucleation and growth, inducing a smoother anode/electrolyte interface compared with the pristine electrolyte. With 1 wt% Mg(TFSI)2 in the PEO-LiTFSI electrolyte, the Mg-modified electrolyte enabled the Li/Li symmetric cells with cycling performance of over 1700 and 1400 h at current densities of 0.1 and 0.2 mA cm−2, respectively. Moreover, the full LFP/Li cells using the novel Mg-modified electrolyte delivered a cycling lifespan of over 450 cycles with negligible capacity loss." @default.
- W3042247998 created "2020-07-23" @default.
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- W3042247998 date "2021-04-01" @default.
- W3042247998 modified "2023-10-15" @default.
- W3042247998 title "In-situ construction of a Mg-modified interface to guide uniform lithium deposition for stable all-solid-state batteries" @default.
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- W3042247998 doi "https://doi.org/10.1016/j.jechem.2020.07.009" @default.
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