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- W3042599268 abstract "Detoxification of hexavalent chromium (Cr(VI)) in the environment and development of corresponding new materials and detoxification protocols have actively been studied and applied. Herein, 2,2′:6′,2′'-terpyridine-4′-thiol (STpy) was functionalized on Au nanoparticle (NP)-loaded carbon paper (CP) and indium-tin-oxide (ITO) electrodes (CP-AuNP and ITO-AuNP, respectively), and the photoelectrochemical (PEC) and photocatalytic detoxification of Cr(VI) using the resulting electrodes was investigated by cyclic voltammetry. Density functional theory at the B3LYP/6-31G level was used for geometry optimization, and the electronic energy state calculation was conducted at the TD-SCF/DFT/B3LYP level. For bare CP, ITO, and STpy-modified AuNP electrodes, the reduction potentials of Cr(VI) were around + 0.3, −0.2 V, and + 0.5 V (vs. Ag/AgCl), respectively. The PEC and photocatalytic Cr(VI) reduction performance of CP-AuNP was significantly improved upon STpy functionalization. Thus, these newly developed functionalized systems can provide very useful information for further improving the detoxification performances for various hazardous metals." @default.
- W3042599268 created "2020-07-23" @default.
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- W3042599268 date "2020-12-01" @default.
- W3042599268 modified "2023-09-24" @default.
- W3042599268 title "Photoelectrochemical and photocatalytic detoxification of Cr(VI) to Cr(III) over terpyridine-derivatized Au nanoparticles on carbon paper and indium-tin-oxide electrodes" @default.
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- W3042599268 doi "https://doi.org/10.1016/j.cej.2020.126266" @default.
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