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- W3042780072 abstract "A non-conjugated polymer acceptor PF1-TS4 was firstly synthesized by embedding a thioalkyl segment in the mainchain, which shows excellent photophysical properties on par with a fully conjugated polymer, with a low optical band gap of 1.58 eV and a high absorption coefficient >105 cm−1, a high LUMO level of −3.89 eV, and suitable crystallinity. Matched with the polymer donor PM6, the PF1-TS4-based all-PSC achieved a power conversion efficiency (PCE) of 8.63 %, which is ≈45 % higher than that of a device based on the small molecule acceptor counterpart IDIC16. Moreover, the PF1-TS4-based all-PSC has good thermal stability with ≈70 % of its initial PCE retained after being stored at 85 °C for 180 h, while the IDIC16-based device only retained ≈50 % of its initial PCE when stored at 85 °C for only 18 h. Our work provides a new strategy to develop efficient polymer acceptor materials by linkage of conjugated units with non-conjugated thioalkyl segments." @default.
- W3042780072 created "2020-07-23" @default.
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- W3042780072 date "2020-08-31" @default.
- W3042780072 modified "2023-10-15" @default.
- W3042780072 title "A Non‐Conjugated Polymer Acceptor for Efficient and Thermally Stable All‐Polymer Solar Cells" @default.
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- W3042780072 doi "https://doi.org/10.1002/anie.202005662" @default.
- W3042780072 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7692906" @default.
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