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- W3043151391 abstract "In this study, Pt nanoclusters with small sizes (~1.8 nm) is designed and loaded onto the inner surface of hollow nano-TiO2 through combining polymer anchoring and photochemical solid-phase reduction strategy. The N-doped mesoporous carbon derived from the polymer is beneficial for the exposure of Pt sites and stabilization of Pt nanoclusters (~1.8 nm), and supplying more active N-sites. More importantly, the pore structure of the N-doped mesoporous carbon layer prepared by air-etching method contributes to the diffusion of reactants/products and exposure of more active Pt sites to promote surface reactions. The as-prepared C/[email protected]2-3% with 0.54 wt% of Pt shows the largest total pore volume (0.46 cm3 g−1) with an average pore size of ~3 nm, and its catalytic activity is greatly improved with a H2 evolution rate of 9086 μmol h−1 g−1, which is about 48 and 96 times that of bare hollow nano-TiO2 and P25, respectively. In addition, the as-prepared C/[email protected]2-3% shows good durability in a 40-h cyclic test." @default.
- W3043151391 created "2020-07-23" @default.
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- W3043151391 date "2020-09-01" @default.
- W3043151391 modified "2023-10-17" @default.
- W3043151391 title "N-doped porous carbon-stabilized Pt in hollow nano-TiO2 with enhanced photocatalytic activity" @default.
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- W3043151391 doi "https://doi.org/10.1016/j.ijhydene.2020.06.275" @default.
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