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- W3043442824 abstract "Designing efficient non-precious electrocatalysts to facilitate overall water splitting is crucial and highly desirable but remains challenging. In this study, we synthesized nitrogen-doped carbon-decorated [email protected] yolk-shelled micro-polyhedras (denoted as [email protected]/NC YSMPs) via the phosphorization of [email protected] Prussian blue analogues YSMPs. The yolk-shelled construction and nitrogen-doped carbon matrix can effectively reduce the degree of CoP agglomeration, which is beneficial for increasing the specific surface area and active sites of the catalysts. The synergistic effect of yolk-shelled structure and nigtrogen-doped carbon matrix also optimizes the electronic structure and enhances the electrocatalytic activity of [email protected]/NC YSMPs. In an alkaline electrolyte, the overpotentials of hydrogen evolution reaction and oxygen evolution reaction only need 141 and 238 mV, respectively, to drive the current density of 10 mA cm−2. When a two-electrode water splitting device was conducted with the as-prepared catalyst, it required only a low cell voltage of 1.68 V to achieve a current density of 10 mA cm−2 and displayed outstanding stability over 20 h. This work offers insights into the facile, controllable synthesis strategy of various non-precious metal nanomaterials for high-efficiency water splitting electrocatalysis." @default.
- W3043442824 created "2020-07-23" @default.
- W3043442824 creator A5014362331 @default.
- W3043442824 creator A5014575317 @default.
- W3043442824 creator A5016988979 @default.
- W3043442824 creator A5058219319 @default.
- W3043442824 creator A5065252871 @default.
- W3043442824 date "2021-01-01" @default.
- W3043442824 modified "2023-10-14" @default.
- W3043442824 title "Nitrogen-doped carbon-decorated yolk-shell CoP@FeCoP micro-polyhedra derived from MOF for efficient overall water splitting" @default.
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- W3043442824 doi "https://doi.org/10.1016/j.cej.2020.126312" @default.
- W3043442824 hasPublicationYear "2021" @default.
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