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• W3043660198 abstract "We report for the first time cyclic phosphine-free “head to tail” N,N,N pincer-like (pincer complexes mimicking) N-(pyrimidin-2-yl)-1,2-azole-3-carboxamide Pd(II) complexes with deprotonated amide groups as high-turnover catalysts (TON up to 106, TOF up to 1.2 × 107 h–1) for cross-coupling reactions on the background of up to quantitative yields under Green Chemistry conditions. The potency of the described catalyst family representatives was demonstrated in Suzuki–Miyaura, Mizoroki–Heck, and Sonogashira reactions on industrially practical examples. Corresponding ligands could be synthesized based on readily available reagents through simple chemical transformations. Within the complex structures, a highly unusual 1,3,5,7-tetraza-2,6-dipalladocane frame could be observed." @default.
• W3043660198 created "2020-07-23" @default.
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• W3043660198 date "2020-07-20" @default.
• W3043660198 modified "2023-10-18" @default.
• W3043660198 title "Mimics of Pincer Ligands: An Accessible Phosphine-Free <i>N</i>-(Pyrimidin-2-yl)-1,2-azole-3-carboxamide Framework for Binuclear Pd(II) Complexes and High-Turnover Catalysis in Water" @default.
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• W3043660198 doi "https://doi.org/10.1021/acs.inorgchem.0c01035" @default.
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• W3043660198 hasPublicationYear "2020" @default.
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