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- W3043816411 abstract "Abstract The practical application of Li–S batteries demands low cell balance (Li capacity /S capacity ), which involves uniform Li growth, restrained shuttle effect, and fast redox reaction kinetics of S species simultaneously. Herein, with the aid of W 2 C nanocrystals, a freestanding 3D current collector is applied as both Li and S hosts owing to its lithiophilic and sulfilic property. On the one hand, the highly conductive W 2 C can reduce Li nucleation overpotentials, thus guiding uniform Li nucleation and deposition to suppress Li dendrite growth. On the other hand, the polar W 2 C with catalytic effect can enhance the chemisorption affinity to lithium polysulfides (LiPSs) and guarantee fast redox kinetics to restrain S species in cathode region and promote the utilization of S. Surprisingly, a full Li–S battery with ultralow cell balance of 1.5:1 and high sulfur loading of 6.06 mg cm −2 shows obvious redox plateaus of S and maintains high reversible specific capacity of 1020 mAh g −1 (6.2 mAh cm −2 ) after 200 cycles. This work may shed new sights on the facile design of full Li–S battery with low excessive Li supply." @default.
- W3043816411 created "2020-07-23" @default.
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- W3043816411 date "2020-10-27" @default.
- W3043816411 modified "2023-10-16" @default.
- W3043816411 title "A Full Li–S Battery with Ultralow Excessive Li Enabled via Lithiophilic and Sulfilic W <sub>2</sub> C Modulation" @default.
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- W3043816411 doi "https://doi.org/10.1002/chem.202002822" @default.
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