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- W3043886507 abstract "Nanoplasmonic hydrogen sensors are predicted to play a key role in safety systems of the emerging hydrogen economy. Pd nanoparticles are the active material of choice for sensor prototype development due to their ability to form a hydride at ambient conditions, which creates the optical contrast. Here, we introduce plasmonic hydrogen sensors made from a thermoplastic nanocomposite material, that is, a bulk material that can be molded with standard plastic processing techniques, such as extrusion and three-dimensional (3D) printing, while at the same time being functionalized at the nanoscale. Specifically, our plasmonic plastic is composed of hydrogen-sensitive and plasmonically active Pd nanocubes mixed with a poly(methyl methacrylate) matrix, and we optimize it by characterization from the atomic to the macroscopic level. We demonstrate melt-processed deactivation-resistant plasmonic hydrogen sensors, which retain full functionality even after 50 weeks. From a wider perspective, we advertise plasmonic plastic nanocomposite materials for application in a multitude of active plasmonic technologies since they provide efficient scalable processing and almost endless functional material design opportunities via tailored polymer–colloidal nanocrystal combinations." @default.
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- W3043886507 date "2020-07-20" @default.
- W3043886507 modified "2023-09-30" @default.
- W3043886507 title "Bulk-Processed Pd Nanocube–Poly(methyl methacrylate) Nanocomposites as Plasmonic Plastics for Hydrogen Sensing" @default.
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- W3043886507 doi "https://doi.org/10.1021/acsanm.0c01907" @default.
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