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- W3044079931 abstract "To address a challenge for decoration of noble metal nanoparticles (NMNPs)-shell on conducting polymer nanofiber (CPNF) electrodes (i.e. NMNP-shell/CPNF-core electrodes) for boosting electrochemical performances, a two-step strategy comprising chemical pre-deposition and electrochemical deposition is designed. The strategy shows a high universality in terms of the diversity of NMNP-shell elements (single-element: AgNP-shell, AuNP-shell, PtNP-shell, PdNP-shell; multi-element: Au/Pt/PdNP-shell) and the independence of conductive substrates of electrodes. The shells are composed of high-density NMNPs and have strong adhesion to CPNF-cores. It is demonstrated that in response to a specific applied electrical stimulus, the resulting low doping level of CPNFs facilitates the generation of high-density nucleation sites (small NMNPs) by chemical pre-deposition (as high capability of electron transfer and low resistance to electron transfer from CP chains to NM ions), which is indispensable for the formation of NMNP-shells on CPNF-cores by electrochemical deposition. The decoration of NMNP-shells can significantly enhance the electrochemical performances of CPNF electrodes. Moreover, the great practicality and reliability of NMNP-shell/CPNF-core electrodes in use as an electrocatalytic platform are confirmed. This universal strategy opens up a new avenue to construct high-dimension shell/core-nanostructured electrodes." @default.
- W3044079931 created "2020-07-29" @default.
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- W3044079931 date "2020-08-11" @default.
- W3044079931 modified "2023-10-14" @default.
- W3044079931 title "A universal strategy: Rational construction of noble metal nanoparticle-shell/conducting polymer nanofiber-core electrodes with enhanced electrochemical performances" @default.
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- W3044079931 doi "https://doi.org/10.1088/1361-6528/aba7e3" @default.
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