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- W3044086254 abstract "Mechanochemical activation is of particular significance in the field of sustainable chemistry. This technique can transform mechanical energy into a chemical reaction under solvent-free conditions, while it has rarely been used in the preparation of near-infrared (NIR) luminescent materials. Here, an NIR luminescent complex with a homogeneous shuttlelike morphology was designed and synthesized through a facile mechanochemical process at room temperature. The successful coordination of Yb3+ with symmetrical terpyridine units and 2-thenoyltrifluoroacetonate synergistically allows the obtained Yb3+ ternary complex to reveal remarkable improvement in the NIR luminescent behavior and thermal-resistant performance compared with the mononuclear complex, Yb(tta)3·3H2O. This enhancement mainly benefits from the removal of water molecules in the first coordination sphere of Yb3+ through the introduction of terpyridines, thus preventing the diffusion of water molecules to Yb3+ complexes, and driving the formation of the Yb3+ complex with more effective coordination number and enhanced the NIR luminescence. This provided a promising environmentally friendly strategy to synthesize highly NIR luminescence materials for eliminating the influence of harmful organic solvents." @default.
- W3044086254 created "2020-07-29" @default.
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- W3044086254 date "2020-07-21" @default.
- W3044086254 modified "2023-09-25" @default.
- W3044086254 title "Enhanced Near-IR Luminescence and Thermal-Resistant Properties of Yb(III) Complexes Under Solvent-Free Mechanochemical Conditions" @default.
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- W3044086254 doi "https://doi.org/10.1021/acssuschemeng.0c00897" @default.
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